2024-03-28T10:00:13Z
https://repository.dl.itc.u-tokyo.ac.jp/oai
oai:repository.dl.itc.u-tokyo.ac.jp:00000718
2022-12-19T03:41:46Z
6:169:170
9:10:11
Exciton diffusion, end quenching, and exciton-exciton annihilation in individual air-suspended carbon nanotubes
Ishii, A.
2699
Yoshida, M.
2700
Kato, Y. K.
2701
Luminescence properties of carbon nanotubes are strongly affected by exciton diffusion, which plays an important role in various nonradiative decay processes. Here we perform photoluminescence microscopy on hundreds of individual air-suspended carbon nanotubes to elucidate the interplay between exciton diffusion, end quenching, and exciton-exciton annihilation processes. A model derived from random-walk theory as well as Monte Carlo simulations are utilized to analyze nanotube length dependence and excitation power dependence of emission intensity. We have obtained the values of exciton diffusion length and absorption cross section for different chiralities, and diameter-dependent photoluminescence quantum yields have been observed. The simulations have also revealed the nature of a one-dimensional coalescence process, and an analytical expression for the power dependence of emission intensity is given.
journal article
American Physical Society
2015-03-19
application/pdf
Physical Review B
12
91
2469-9969
https://repository.dl.itc.u-tokyo.ac.jp/record/718/files/PhysRevB.91.125427.pdf
eng